Advanced Crystallography

Twinning, Miller indices, crystal habits, crystal forms, point groups, and crystal growth mechanisms.

crystallography twinning miller-indices point-groups crystal-habit

Introduction

Advanced crystallography builds on the foundation of crystal systems to explore
how crystals grow, twin, and develop their characteristic forms. Understanding
these concepts is essential for interpreting inclusion patterns, growth features,
and crystal morphology.

The FGA Diploma requires ability to draw common crystal habits and understand
twinning patterns—these visual skills are tested in examinations.

Miller Indices

Miller indices describe the orientation of crystal faces relative to crystallographic
axes. They are fundamental to describing crystal forms and understanding
morphology.

Three-Index Notation {hkl}

For cubic, tetragonal, orthorhombic, monoclinic, and triclinic systems:

  1. Determine where face intercepts each axis (a, b, c)
  2. Take reciprocals of these intercepts
  3. Clear fractions to get smallest integers
  4. Enclose in braces {hkl} for a form (set of symmetrically equivalent faces)
  5. Use parentheses (hkl) for a single specific face

Example: Face intercepts a at 1, b at 2, c at ∞

  • Reciprocals: 1/1, 1/2, 1/∞ = 1, 0.5, 0
  • Clear fractions: multiply by 2 → 2, 1, 0
  • Miller index: (210)
Common Cubic Forms

Four-Index Notation {hkil}

For hexagonal and trigonal systems, four-index (Miller-Bravais) notation uses
three horizontal axes (a₁, a₂, a₃) at 120° plus vertical c-axis:

  • h + k + i = 0 (always; i is redundant but clarifies symmetry)
  • Negative indices shown with bar: 1̄ or written as -1

Example: {10-10} = {101̄0} = hexagonal prism faces

Common hexagonal/trigonal forms:

  • {0001} - Basal pinacoid (top and bottom)
  • {10-10} - Hexagonal prism
  • {10-11} - Hexagonal dipyramid
  • {11-20} - Second-order prism

Crystal Forms

A crystal form is a set of faces that are equivalent by symmetry. Forms can be
open (don't enclose space alone) or closed (can exist independently).

Open vs Closed Forms

Form Combinations

Real crystals typically show multiple forms in combination:

  • Dominant form: Largest faces, determines overall shape
  • Modifying forms: Smaller faces, truncate edges/corners
  • CDL notation: {111}@1.0 + {100}@1.3 describes relative development

Example: Diamond often shows {111} octahedron with {100} cube faces
truncating corners.

Twinning

Twinning occurs when two or more crystals share some lattice points but have
different orientations. Twins can form during growth, transformation, or
mechanical stress.

Types of Twins

Type Description Examples
Contact twins Share a plane; mirror reflection Spinel twin, quartz Brazil twin
Penetration twins Interpenetrate; share a line/point Fluorite, staurolite cross
Polysynthetic (lamellar) Multiple parallel thin twins Plagioclase, labradorite
Cyclic twins Three or more parts around axis Chrysoberyl trillings, rutile

Twin Laws

A twin law describes the geometric relationship between twin parts:

  • Twin plane: Mirror plane relating the parts
  • Twin axis: Rotation axis (typically 180°)
  • Contact vs penetration: Whether parts share plane or interpenetrate

Common twin laws include spinel law {111}, Brazil law in quartz, and
Carlsbad law in orthoclase.

Important Twins in Gemmology

Diagnostic Twins by Species
Mineral Twin Type Appearance Significance
Spinel Contact octahedral Flattened triangular plates Characteristic habit
Chrysoberyl Cyclic (trillings) Six-rayed star shape Common; pseudohexagonal
Quartz Brazil law Alternating right/left zones Optical effects
Quartz Dauphiné law No visible twin plane Detected by etch figures
Rutile Cyclic (geniculae) Knee-shaped twins Common at 60° or 90°
Fluorite Penetration Interpenetrating cubes Characteristic
Staurolite Cross penetration 60° or 90° crosses Fairy crosses
Feldspar Polysynthetic Parallel striations Twinning lamellae

Twinning Effects

Crystal Habits

Crystal habit describes the overall shape a mineral typically assumes. The same
mineral can show different habits depending on growth conditions.

Common Habit Terms

Term Description Examples
Prismatic Elongated parallel to c-axis Tourmaline, beryl
Tabular Flat, plate-like Mica, topaz
Equant Roughly equal dimensions Garnet, diamond
Acicular Needle-like Rutile, actinolite
Bladed Flat, elongated like knife blade Kyanite
Fibrous Thread-like aggregates Asbestos, tiger's eye
Massive No visible crystal faces Jadeite, nephrite
Botryoidal Grape-like rounded masses Malachite, chalcedony

Habit Variations

The same mineral may show different habits due to:

  • Growth rate: Fast growth → elongated; slow growth → equant
  • Temperature: Higher temperatures often favour specific faces
  • Impurities: Can block growth on certain faces
  • Available space: Constrained environments modify shape
  • Supersaturation: Affects relative face development

Species-Specific Habits

Typical Crystal Shapes

  • Diamond: octahedron, dodecahedron
  • Corundum: barrel-shaped, tabular hexagonal
  • Beryl: hexagonal prism with flat termination
  • Quartz: hexagonal prism with pyramid
  • Tourmaline: triangular prism
  • Topaz: orthorhombic prism with dome
  • Spinel: octahedron (often twinned)
  • Garnet: dodecahedron or trapezohedron

Atypical Habits

  • Diamond: cube (rare), flat triangular macles
  • Corundum: bipyramidal, prismatic
  • Beryl: etched, tapered
  • Quartz: sceptre, skeletal, Japan twin
  • Tourmaline: slender prismatic, massive
  • Spinel: cube (rare)
  • Garnet: massive, granular

The 32 Point Groups

Point groups (crystal classes) describe the symmetry elements present at a point.
Each crystal system contains multiple point groups.

Point Group Notation

Hermann-Mauguin notation describes symmetry elements:

  • Numbers (2, 3, 4, 6): Rotation axes (fold symmetry)
  • m: Mirror plane
  • Bar notation (-1, -3, -4, -6): Rotoinversion axes
  • Combination (4/m): Axis perpendicular to mirror
Cubic System Point Groups
Hexagonal and Trigonal Point Groups

Crystal Growth

Understanding crystal growth explains many inclusion patterns, zoning features,
and quality characteristics observed in gems.

Growth Mechanisms

Crystals grow by atoms/molecules attaching to energetically favourable sites:

  • Layer growth: Atoms add to stepped surfaces
  • Screw dislocation growth: Spiral growth patterns
  • Dendritic growth: Fast growth → branching patterns
  • Skeletal growth: Edges grow faster than faces

Growth Features

Feature Cause Example
Colour zoning Changing conditions during growth Sapphire, tourmaline
Phantom crystals Growth interruption and resumption Quartz phantoms
Growth tubes Inclusions elongated by growth Tourmaline, beryl
Negative crystals Fluid-filled voids with crystal shape Spinel, quartz
Hourglass zoning Different impurity uptake on faces Synthetic corundum
Striae Subtle parallel growth lines Tourmaline, beryl

Natural vs Synthetic Growth

Growth features help distinguish natural from synthetic gems:

  • Natural: Irregular zoning, varied inclusion suites, geological timeframe
  • Flame fusion: Curved striae from rotating growth
  • Flux growth: Flux inclusions, metallic platelets
  • Hydrothermal: Chevron zoning, seed plates

Crystal Drawing

CDL Crystal Examples

The Crystal Description Language (CDL) provides a notation for describing crystal
morphology. These examples show common gem crystal shapes.

Cubic Examples

Diamond octahedron with cube truncations:

Trigonal Examples

Quartz prism with rhombohedral terminations:

Hexagonal Examples

Beryl (emerald) hexagonal prism with pinacoid: